Pressure tuning of the thermal conductivity of the layered muscovite crystal

Wen- Pin Hsieh, Bin Chen, Jie Li, Pawel Keblinski, and David G. Cahill

Accepted Wednesday Nov 04, 2009

The physics of heat conduction in layered, anisotropic crystals is probed by measurements of the cross-plane elastic constant C33 and thermal conductivity \Lambda of muscovite mica as a function of hydrostatic pressure. Picosecond interferometry and time-domain thermoreflectance provide high precision measurements of C33 and \Lambda, respectively, of micron-sized samples within a diamond anvil cell; \Lambda changes from the anomalously low value of 0.46 W m-1 K-1 at ambient pressure to a value more typical of oxides crystals with large unit cells, 6.6 W m-1 K-1, at P=24 GPa. Most of the pressure dependence of \Lambda can be accounted for by the pressure dependence of the cross-plane sound velocities.