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Phys. Rev. B 80, 075431 (2009) [5 pages]

Angle-resolved photoemission study of the graphite intercalation compound KC8: A key to graphene

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A. Grüneis1,2,*, C. Attaccalite3, A. Rubio3,4, D. V. Vyalikh5, S. L. Molodtsov5, J. Fink2,6, R. Follath6, W. Eberhardt6, B. Büchner2, and T. Pichler1
1Faculty of Physics, Vienna University, Strudlhofgasse 4, 1090 Wien, Austria
2IFW Dresden, P.O. Box 270116, D-01171 Dresden, Germany
3Nano-Bio Spectroscopy Group and ETSF Scientific Development Centre, Dpto. Física de Materiales, Universidad del País Vasco, Centro de Física de Materiales CSIC-UPV/EHU-MPC and DIPC, Av. Tolosa 72, E-20018 San Sebastián, Spain
4Fritz-Haber-Institute of the Max Planck Society, Theory Department, Faradayweg 4-6, D-14195 Berlin-Dahlem, Germany
5Institut für Festkörperphysik, TU Dresden, Mommsenstrasse 13, D-01069 Dresden, Germany
6Helmholtz-Zentrum Berlin, Albert-Einstein-Strasse 15, 12489 Berlin, Germany

Received 23 December 2008; revised 29 June 2009; published 27 August 2009

See accompanying Physics Synopsis

Electrons in isolated graphene layers are a two-dimensional gas of massless Dirac Fermions. In realistic devices, however, the electronic properties are modified by elastic deformations, interlayer coupling and substrate interaction. Here, we unravel the electronic structure of noninteracting, doped graphene layers by revisiting the stage one graphite intercalation compound KC8. To this end we apply angle-resolved photoemission spectroscopy and ab initio calculations. The full experimental dispersion is in excellent agreement with calculations of doped graphene once electron correlations are included at the GW level (Greens function G of the Coulomb interaction W). This highlights that KC8 has negligible interlayer coupling allowing us to access the full experimental Dirac cone.

© 2009 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.80.075431
DOI:
10.1103/PhysRevB.80.075431
PACS:
71.18.+y, 79.60.−i

*Corresponding author; ag3@biela.ifw-dresden.de