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Phys. Rev. B 79, 245405 (2009) [9 pages]

Aperiodic and modulated Pb thin films on fivefold icosahedral Al-Cu-Fe and Al(111): Tailoring the structure of Pb

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Th. Deniozou, J. Ledieu, and V. Fournée
Institut Jean Lamour, UMR 7198 CNRS - Nancy Université - UPV Metz, Ecole des Mines de Nancy, Parc de Saurupt, CS 14234, 54042 Nancy Cedex, France

D. M. Wu and T. A. Lograsso
Ames Laboratory, Iowa State University, Ames, Iowa 50011, USA

H. I. Li and R. D. Diehl
Department of Physics, Pennsylvania State University, University Park, Pennsylvania 16802, USA

Received 16 February 2009; published 5 June 2009

We report on the growth of Pb thin films deposited either on the Al-rich fivefold surface of the icosahedral Al-Cu-Fe quasicrystal or on the (111) surface of fcc Al. On the quasicrystalline substrate, the diffusion length of Pb adatoms is short due to heterogeneous nucleation that enforces a quasiperiodic structure in the monolayer. On the Al(111) substrate, the mobility of Pb adatoms is high and the interaction with the substrate is flatter, leading to the formation of a (√31×√31)R8.95° higher-order commensurate structure. This moiré structure propagates up to the highest coverages investigated.

© 2009 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.79.245405
DOI:
10.1103/PhysRevB.79.245405
PACS:
68.37.Ef, 68.35.Rh, 71.23.Ft, 71.15.Mb