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Phys. Rev. B 79, 224433 (2009) [17 pages]

Orbitally induced string formation in the spin-orbital polarons

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Krzysztof Wohlfeld1,2, Andrzej M. Oleś1,2, and Peter Horsch1
1Max-Planck-Institut für Festkörperforschung, Heisenbergstrasse 1, D-70569 Stuttgart, Germany
2Marian Smoluchowski Institute of Physics, Jagellonian University, Reymonta 4, PL-30059 Kraków, Poland

Received 28 February 2009; revised 12 May 2009; published 29 June 2009

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We study the spectral function of a single hole doped into the ab plane of the Mott insulator LaVO3, with antiferromagnetic (AF) spin order of S=1 spins accompanied by alternating orbital (AO) order of active {dyz,dzx} orbitals. Starting from the respective t-J model, with spin-orbital superexchange and effective three-site hopping terms, we derive the polaron Hamiltonian and show that a hole couples simultaneously to the collective excitations of the AF/AO phase, magnons, and orbitons. Next, we solve this polaron problem using the self-consistent Born approximation and find a stable quasiparticle solution—a spin-orbital polaron. We show that the spin-orbital polaron resembles the orbital polaron found in eg systems, as e.g., in K2CuF4 or (to some extent) in LaMnO3, and that the hole may be seen as confined in a stringlike potential. However, the spins also play a crucial role in the formation of this polaron—we explain how the orbital degrees of freedom: (i) confine the spin dynamics acting on the hole as the classical Ising spins and (ii) generate the string potential which is of the joint spin-orbital character. Finally, we discuss the impact of the results presented here on the understanding of the phase diagrams of the lightly doped cubic vanadates.

© 2009 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.79.224433
DOI:
10.1103/PhysRevB.79.224433
PACS:
71.10.Fd, 72.10.Di, 72.80.Ga, 79.60.−i