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Phys. Rev. B 78, 054529 (2008) [6 pages]

Doping evolution of antiferromagnetic order and structural distortion in LaFeAsO1−xFx

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Q. Huang1, Jun Zhao2, J. W. Lynn1, G. F. Chen3, J. L. Luo3, N. L. Wang3, and Pengcheng Dai2,4,*
1NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899-6102, USA
2Department of Physics and Astronomy, The University of Tennessee, Knoxville, Tennessee 37996-1200, USA
3Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, P.O. Box 603, Beijing 100080, People’s Republic of China
4Neutron Scattering Science Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831-6393, USA

Received 17 July 2008; revised 26 July 2008; published 28 August 2008

We use neutron scattering to study the structural distortion and antiferromagnetic (AFM) order in LaFeAsO1−xFx as the system is doped with fluorine (F) to induce superconductivity. In the undoped state, LaFeAsO exhibits a structural distortion, changing the symmetry from tetragonal (space group P4/nmm) to orthorhombic (space group Cmma) at 155 K, and then followed by an AFM order at 137 K. Doping the system with F gradually decreases the structural distortion temperature, but suppresses the long range AFM order before the emergence of superconductivity. Therefore, while superconductivity in these Fe oxypnictides can survive in either the tetragonal or the orthorhombic crystal structure, it competes directly with static AFM order.

© 2008 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.78.054529
DOI:
10.1103/PhysRevB.78.054529
PACS:
75.25.+z, 75.50.Ee, 25.40.Dn, 75.30.Fv

*daip@ornl.gov