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Phys. Rev. B 78, 224518 (2008) [5 pages]

Phonon dynamics in Sr0.6K0.4Fe2As2 and Ca0.6Na0.4Fe2As2 from neutron scattering and lattice-dynamical calculations

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R. Mittal1,2, Y. Su1, S. Rols3, M. Tegel4, S. L. Chaplot2, H. Schober3, T. Chatterji5, D. Johrendt4, and Th. Brueckel1,6
1Juelich Centre for Neutron Science, IFF, Forschungszentrum Juelich, Outstation at FRM II, Lichtenbergstrasse 1, D-85747 Garching, Germany
2Solid State Physics Division, Bhabha Atomic Research Centre, Trombay, Mumbai 400 085, India
3Institut Laue-Langevin, BP 156, 38042 Grenoble Cedex 9, France
4Department Chemie und Biochemie, Ludwig-Maximilians-Universitaet Muenchen, Butenandtstrasse 5-13 (Haus D), D-81377 Muenchen, Germany
5Juelich Centre for Neutron Science, Forschungszentrum Juelich, Outstation at Institut Laue-Langevin, BP 156, 38042 Grenoble Cedex 9, France
6Institut fuer Festkoerperforschung, Forschungszentrum Juelich, D-52425 Juelich, Germany

Received 24 October 2008; revised 17 November 2008; published 19 December 2008

We report inelastic neutron scattering measurements of the phonon density of states of superconducting Sr0.6K0.4Fe2As2 (Tc=32 K) and Ca0.6Na0.4Fe2As2 (Tc=21 K). Compared with the parent compound BaFe2As2 doping affects mainly the lower and intermediate frequency part of the vibrations. Mass effects and lattice contraction cannot solely explain these changes. Softening of phonon modes below 10 meV has been observed in both samples on cooling from 300 to 140 K. In the Ca-doped compound the softening amounts to about 1 meV while for the Sr-doped compound the softening is about 0.5 meV. There is no appreciable change in the phonon density of states on crossing Tc.

© 2008 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.78.224518
DOI:
10.1103/PhysRevB.78.224518
PACS:
74.25.Kc, 78.70.Nx, 63.20.−e