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Phys. Rev. B 78, 180504(R) (2008) [4 pages]

Strong coupling between magnetic and structural order parameters in SrFe2As2

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A. Jesche1, N. Caroca-Canales1, H. Rosner1, H. Borrmann1, A. Ormeci1, D. Kasinathan1, H. H. Klauss2, H. Luetkens3, R. Khasanov3, A. Amato3, A. Hoser4, K. Kaneko1,5, C. Krellner1, and C. Geibel1,*
1Max Planck Institute for Chemical Physics of Solids, D-01187 Dresden, Germany
2IFP, TU-Dresden, D-01069 Dresden, Germany
3Laboratory for Muon-Spin Spectroscopy, Paul-Scherrer-Institute, CH-5232 Villigen, Switzerland
4Hahn-Meitner-Institute, D-14109 Berlin, Germany
5Advanced Science Research Center, Japan Atomic Energy Agency, Tokai, Ibaraki 319-1195, Japan

Received 4 July 2008; revised 26 September 2008; published 13 November 2008

X-ray and muon spin-relaxation experiments performed on SrFe2As2 polycrystals confirm a sharp first-order transition at T0=205 K corresponding to an orthorhombic phase distortion and to a commensurate antiferromagnetic Fe ordering with a larger distortion and larger size of the ordered moment than reported for BaFe2As2. The structural and the magnetic order parameters present a remarkable similarity in their temperature dependence from T0 down to low temperatures, showing that both phenomena are intimately connected. Accordingly, the size of the ordered Fe moments scales with the lattice distortion when going from SrFe2As2 to BaFe2As2. Full-potential band-structure calculations confirm that the columnar magnetic order with propagation vector (1,0,1) and the orthorhombic lattice distortion are intrinsically tied to each other.

© 2008 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.78.180504
DOI:
10.1103/PhysRevB.78.180504
PACS:
71.20.Lp, 74.70.Dd, 75.30.Fv

*geibel@cpfs.mpg.de