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Phys. Rev. B 77, 172406 (2008) [4 pages]

Detection of weak emergent broken-symmetries of the kagome antiferromagnet by Raman spectroscopy

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O. Cépas1, J. O. Haerter1,2, and C. Lhuillier1
1Laboratoire de Physique Théorique de la Matière Condensée, UMR 7600 CNRS, Université Pierre-et-Marie-Curie, Paris VI, 75252 Paris cedex 05, France
2Department of Physics, University of California, Santa Cruz, California 95064, USA

Received 1 February 2008; revised 4 April 2008; published 16 May 2008

We show that the magnetic Raman response of a spin liquid is independent of the polarizations of the light for triangular symmetries. In contrast, a ground state that has a broken-symmetry shows characteristic oscillations when the polarizations are rotated. This would allow one to detect weak broken-symmetries and emergent order parameters. We focus on the kagome antiferromagnet wherein no conventional long-range order has been found so far and present the Raman cross section of a spin liquid and a valence bond crystal by using a random phase approximation.

© 2008 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.77.172406
DOI:
10.1103/PhysRevB.77.172406
PACS:
75.10.Jm, 75.40.Gb