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Phys. Rev. B 76, 104515 (2007) [8 pages]

Magnetic structure of Sm2IrIn8 determined by x-ray resonant magnetic scattering

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C. Adriano1,*, R. Lora-Serrano1, C. Giles1, F. de Bergevin2, J. C. Lang3, G. Srajer3, C. Mazzoli2, L. Paolasini2, and P. G. Pagliuso1
1Instituto de Física “Gleb Wataghin,” UNICAMP, 13083-970 Campinas-SP, Brazil
2European Synchrotron Radiation Facility, Grenoble 38043, France
3Advanced Photon Source, Argonne National Laboratory, Argonne, Illinois 60439, USA

Received 22 April 2007; published 21 September 2007

The magnetic structure of the intermetallic antiferromagnet Sm2IrIn8 was determined using x-ray resonant magnetic scattering. Below TN=14.2 K, Sm2IrIn8 has a commensurate antiferromagnetic structure with a propagation vector η⃗=(1∕2,0,0). The Sm magnetic moments lie in the ab plane and are rotated roughly 18° away from the a axis. The magnetic structure of this compound was obtained by measuring the strong dipolar resonant peak whose enhancement was of over 2 orders of magnitude at the L2 edge. At the L3 edge, both quadrupolar and dipolar features were observed in the energy line shape. The magnetic structure and properties of Sm2IrIn8 are found to be consistent with the general trend already seen for the Nd-, Tb-, and the Ce-based compounds from the RmMnIn3m+2n family (R=rare earth; M=Rh or Ir; m=1,2; n=0,1), where the crystalline electrical field effects determine the direction of magnetic moments and the TN evolution in the series. The measured Néel temperature for Sm2IrIn8 is slightly suppressed when compared to the TN of the parent cubic compound SmIn3.

© 2007 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.76.104515
DOI:
10.1103/PhysRevB.76.104515
PACS:
71.20.Lp, 75.25.+z, 75.50.Ee, 75.30.−m

*cadriano@ifi.unicamp.br