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Phys. Rev. B 72, 094306 (2005) [5 pages]

Dimensional mismatch of the electron-phonon system and large polaron stability

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Zoran Ivić*
The “Vinča” Institute of Nuclear Sciences, Laboratory for Theoretical and Condensed Matter Physics—020, P.O. Box 522, 11001 Belgrade, Serbia and Montenegro

David W. Brown
University of California, San Diego, CMRR Building, 9500 Gilman Drive, La Jolla, California 92093-0402, USA

Marijana Kirćan
Institut für Theorie der Kondensierten Materie, Universität Karlsruhe, Postfach 6980, 76128 Karlsruhe, Germany

Received 21 February 2005; revised 20 May 2005; published 30 September 2005

We consider the scaling arguments in the adiabatic limit for materials in which one-dimensional (1D) electronic behavior is influenced by a higher-dimensional vibrational system. The system under consideration consists of a collection of widely separated parallel molecular chains, perfectly one dimensional in respect to their electronic characteristics, embedded in a three-dimensional (3D) lattice. We found that dimensional mismatch between electronic subsystem and lattice may seriously affect polaron stability. For the realistic systems with anisotropic phonon spectrum large polaron stability requires that polaron radius cannot exceed some critical value which is of the order of the interchain spacing. Finally, large polaron stability criterion is formulated in dependence of the values of the basic system parameters.

© 2005 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.72.094306
DOI:
10.1103/PhysRevB.72.094306
PACS:
71.38.−k

*Electronic address: zivic@rt270.vin.bg.ac.yu