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Phys. Rev. B 72, 075401 (2005) [13 pages]

Vibrational spectra of amorphous clusters: Universal aspects

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Gurpreet S. Matharoo, Subir K. Sarkar, and Akhilesh Pandey
School of Physical Sciences, Jawaharlal Nehru University, New Delhi 110 067, India

Received 9 February 2005; revised 4 May 2005; published 1 August 2005

We have performed extensive numerical computations on the vibrational spectra of isolated amorphous clusters of medium to large size and containing one or two types of atoms. The interaction potential is also varied to study possible universality. For all the potentials and cluster sizes we find that the cumulative density of states can be described very accurately by the same functional form over a large central region of the spectrum. This functional form contains only one scale of frequency. We also find that the statistical fluctuations of the spectra are described by the Gaussian orthogonal ensemble of random matrices. For the largest clusters this is tested to a very high degree of precision in the central region and to a somewhat lower degree for most of the rest of the spectrum. We put forward a conjecture regarding the domain of the space of local minima of the potential energy function where universality with respect to the density of states function may be expected.

© 2005 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.72.075401
DOI:
10.1103/PhysRevB.72.075401
PACS:
05.45.Mt, 63.50.+x, 61.43.Fs, 24.60.Lz