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Phys. Rev. B 72, 214204 (2005) [9 pages]

Anharmonic versus relaxational sound damping in glasses. I. Brillouin scattering from densified silica

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Evelyne Rat1, Marie Foret2,*, Gladys Massiera1,†, Rémy Vialla2, Masatoshi Arai3, René Vacher2, and Eric Courtens2
1Laboratoire des Verres, UMR 5587 CNRS, Université Montpellier II, F-34095 Montpellier Cedex 5, France
2Laboratoire des Colloïdes, Verres et Nanomatériaux, UMR 5587 CNRS, Université Montpellier II, F-34095 Montpellier Cedex 5, France
3High Intensity Proton Accelerator Project Division, High Energy Accelerator Research Organization, 1-1 Oho, Tsukuba 305-0801, Japan

Received 20 May 2005; revised 16 September 2005; published 9 December 2005

This series discusses the origin of sound damping and dispersion in glasses. In particular, we address the relative importance of anharmonicity versus thermally activated relaxation. In this first article, Brillouin-scattering measurements of permanently densified silica glass are presented. It is found that in this case the results are compatible with a model in which damping and dispersion are only produced by the anharmonic coupling of the sound waves with thermally excited modes. The thermal relaxation time and the unrelaxed velocity are estimated.

© 2005 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.72.214204
DOI:
10.1103/PhysRevB.72.214204
PACS:
78.40.Pg, 63.50.+x, 78.35.+c

*Corresponding author: Marie.Foret@lcvn.univ-montp2.fr

Present address: Laboratoire de Spectrométrie Physique, Université Joseph Fourier, F-38402 Saint Martin d’Hères, France.