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Phys. Rev. B 72, 014428 (2005) [12 pages]

Magnetic properties of pure and Gd-doped EuO probed by NMR

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Arnaud Comment* and Jean-Philippe Ansermet
Department of Physics and Materials Research Laboratory, University of Illinois at Urbana-Champaign, 1110 West Green Street, Urbana, Illinois 61801-3080, USA and Institut de Physique des Nanostructures, Ecole Polytechnique Fédérale de Lausanne, CH-1015 Lausanne-EPFL, Switzerland

Charles P. Slichter
Department of Physics and Materials Research Laboratory, University of Illinois at Urbana-Champaign, 1110 West Green Street, Urbana, Illinois 61801-3080, USA

Heesuk Rho, Clark S. Snow, and S. Lance Cooper
Materials Research Laboratory, University of Illinois at Urbana-Champaign, 104 South Goodwin Ave, Urbana, Illinois 61801-3080, USA

Received 11 October 2004; revised 25 May 2005; published 14 July 2005

An Eu NMR study in the ferromagnetic phase of pure and Gd-doped EuO was performed. A complete description of the NMR line shape of pure EuO allowed for the influence of doping EuO with Gd impurities to be highlighted. The presence of a temperature-dependent static magnetic inhomogeneity in Gd-doped EuO was demonstrated by studying the temperature dependence of the line shapes. The results suggest that the inhomogeneity in 0.6% Gd-doped EuO is linked to colossal magnetoresistance. The measurement of the spin-lattice relaxation times as a function of temperature led to the determination of the value of the exchange integral J as a function of Gd doping. It was found that J is temperature independent and spatially homogeneous for all samples and that its value increases abruptly with increasing Gd doping.

© 2005 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.72.014428
DOI:
10.1103/PhysRevB.72.014428
PACS:
71.30.+h, 75.30.−m, 76.60.−k, 75.50.Pp

*Electronic address: arnaud.comment@epfl.ch

Present address: Department of Physics, Chonbuk National University, Jeonju 561-756, Korea.