Phys. Rev. B 70, 064401 (2004) [12 pages]Dzyaloshinskii-Moriya interactions and adiabatic magnetization dynamics in molecular magnetsReceived 23 December 2003; revised 27 April 2004; published 2 August 2004 A microscopic model of the molecular magnet V15 is used to study mechanisms for the adiabatic change of the magnetization in time-dependent magnetic fields. The effects of the Dzyaloshinskii-Moriya interaction, the most plausible source for the energy-level repulsions that lead to adiabatic changes of the magnetization, are studied in detail. We find that the energy-level repulsions that result from this interaction exhibit a strong dependence on the direction of the applied field. We also discuss the role of magnetic anisotropy in the molecule Mn12-acetate. © 2004 The American Physical Society URL:
http://link.aps.org/doi/10.1103/PhysRevB.70.064401
DOI:
10.1103/PhysRevB.70.064401
PACS:
75.10.Jm, 75.50.Xx, 75.45.+j, 75.50.Ee
|
