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Phys. Rev. B 69, 045114 (2004) [9 pages]

Ultrafast quasiparticle relaxation dynamics in normal metals and heavy-fermion materials

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K. H. Ahn, M. J. Graf, S. A. Trugman, J. Demsar*, R. D. Averitt, J. L. Sarrao, and A. J. Taylor
Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA

Received 11 August 2003; published 30 January 2004

We present a detailed theoretical study of the ultrafast quasiparticle relaxation dynamics observed in normal metals and heavy-fermion materials with femtosecond time-resolved optical pump-probe spectroscopy. For normal metals, a nonthermal electron distribution gives rise to a temperature- (T) independent electron-phonon relaxation time at low temperatures, in contrast to the T-3-divergent behavior predicted by the two-temperature model. For heavy-fermion compounds, we find that the blocking of electron-phonon scattering for heavy electrons within the density-of-states peak near the Fermi energy is crucial to explain the rapid increase of the electron-phonon relaxation time below the Kondo temperature. We propose the hypothesis that the slower Fermi velocity compared to the sound velocity provides a natural blocking mechanism due to energy and momentum-conservation laws.

© 2004 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.69.045114
DOI:
10.1103/PhysRevB.69.045114
PACS:
71.27.+a, 78.47.+p, 71.10.-w

*Present address: “J. Stefan” Institute, Jamova 39, SI-1000, Ljubljana, Slovenia.