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Phys. Rev. B 65, 245325 (2002) [10 pages]

Effects of intervalence band coherences on the coherently coupled heavy-hole–light-hole Stark shift in semiconductor quantum wells

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I. Rumyantsev1, N. H. Kwong2, R. Takayama2, and R. Binder1
1Optical Sciences Center, University of Arizona, Tucson, Arizona 85721
2Cooperative Excitation Project, ERATO, Japan Science and Technology Corporation, Optical Sciences Center, University of Arizona, Tucson, Arizona 85721

Received 25 February 2002; published 24 June 2002

A theoretical study of the coherently coupled heavy-hole–light-hole optical Stark effect in semiconductor quantum wells is presented. Based on a detailed investigation of the various many-body contributions to the Stark shifts, we identify a parameter regime in which the existence of intervalence band coherences (analogous to the nonradiative Raman coherence in three-level atoms) can be inferred from the coherently coupled heavy-hole–light-hole excitonic optical Stark shift. The analysis is performed for the third-order nonlinear optical regime (χ3 regime), and is based on the dynamics-controlled truncation (DCT) formalism. It includes the relevant optical selection rules, excitonic and two-exciton-correlation (e.g., biexcitonic) effects.

© 2002 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.65.245325
DOI:
10.1103/PhysRevB.65.245325
PACS:
78.47.+p, 42.50.Md, 73.21.Fg, 78.67.De