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Phys. Rev. B 65, 014427 (2001) [5 pages]

Structure of nanoscale polaron correlations in La1.2Sr1.8Mn2O7

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B. J. Campbell1,*, R. Osborn1, D. N. Argyriou1, L. Vasiliu-Doloc2,3, J. F. Mitchell1, S. K. Sinha3, U. Ruett1, C. D. Ling1, Z. Islam2,3, and J. W. Lynn4
1Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439
2Department of Physics, Northern Illinois University, DeKalb, Illinois 60115
3Advanced Photon Source, Argonne National Laboratory, Argonne, Illinois 60439
4NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899

Received 6 July 2001; published 11 December 2001

A system of strongly interacting electron-lattice polarons can exhibit charge and orbital order at sufficiently high polaron concentrations. In this study, the structure of short-range polaron correlations in the layered colossal magnetoresistive perovskite manganite La1.2Sr1.8Mn2O7 has been determined by a crystallographic analysis of broad satellite maxima observed in diffuse x-ray and neutron-scattering data. The resulting q(0.3,0,±1) modulation is a longitudinal octahedral-stretch mode, consistent with incommensurate Jahn-Teller-coupled charge-density-wave fluctuations, that implies an unusual orbital-stripe pattern parallel to the 100 directions.

© 2001 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.65.014427
DOI:
10.1103/PhysRevB.65.014427
PACS:
75.30.Vn, 71.30.+h, 71.38.-k, 71.45.Lr

*Electronic address: branton@anl.gov