Phys. Rev. B 64, 100201(R) (2001) [4 pages]Evidence for long-range interactions between rare-earth impurity ions in nanocrystals embedded in amorphous matrices with the two-level systems of the matrix
The low-temperature homogeneous broadening of the electronic transitions of Eu3+ and Pr3+ rare-earth impurity ions in Y2O3 and LaF3 nanocrystals embedded into amorphous materials (polymer and oxyfluoride glass ceramics) was studied with hole-burning and fluorescence line narrowing techniques. It is shown that the homogeneous linewidth is determined by the interaction of the impurity ions contained in the nanocrystals with the two-level systems (TLS’s) of the surrounding glass matrix. A comparison of the experiments with a calculation provides direct evidence for the long-range nature of the interaction with the TLS’s. © 2001 The American Physical Society URL:
http://link.aps.org/doi/10.1103/PhysRevB.64.100201
DOI:
10.1103/PhysRevB.64.100201
PACS:
78.67.-n, 78.67.Bf
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