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Phys. Rev. B 62, 2998–3001 (2000)

Evidence of quantum criticality in the doped Haldane system Y2BaNiO5

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C. Payen, E. Janod, and K. Schoumacker
Institut des Materiaux Jean Rouxel, Universite de Nantes–CNRS, 44322 Nantes Cedex 3, France

C. D. Batista, K. Hallberg, and A. A. Aligia
Centro Atómico Bariloche and Instituto Balseiro, Comisión Nacional de Energía Atómica, 8400 San Carlos de Bariloche, Argentina

Received 13 April 2000; published in the issue dated 1 August 2000

Experimental bulk susceptibility χ(T) and magnetization M(H,T) of the S=1 Haldane chain system doped with nonmagnetic impurities, Y2BaNi1-xZnxO5 (x<~0.08), are analyzed. A numerical calculation for the low-energy spectrum of noninteracting open segments describes well experimental data above 4 K. Below 4 K, we observe power-law behaviors χ(T)T-α and M(H,T)T1-αfα(H/T), with α(<1) depending on the doping concentration x. This observation suggests the appearance of a gapless quantum phase due to a broad distribution of effective couplings between the dilution-induced moments.

© 2000 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.62.2998
DOI:
10.1103/PhysRevB.62.2998
PACS:
75.10.Jm, 75.40.Cx, 75.40.Mg, 75.45.+j