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Phys. Rev. B 61, 1149–1159 (2000)

Quantum spin liquid: The Heisenberg antiferromagnet on the three-dimensional pyrochlore lattice

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Benjamin Canals
Laboratoire de Magnétisme Louis Néel, CNRS, Boîte Postale 166, 38042 Grenoble Cedex 9, France
Max-Planck-Institut für Physik komplexer Systeme, Nöthnitzer Straße 38, D-01187 Dresden, Germany

Claudine Lacroix
Laboratoire de Magnétisme Louis Néel, CNRS, Boîte Postale 166, 38042 Grenoble Cedex 9, France

Received 16 February 1999; revised 20 July 1999; published in the issue dated 1 January 2000

We calculate the correlation functions of the S=1/2 Heisenberg antiferromagnet on the three-dimensional pyrochlore lattice. We use a perturbative expansion in terms of spin blocks. This method is self-controlled by the extracted correlation length. We find that the ground state is a spin-liquid state: the spin-spin correlation functions decay exponentially with distance and the correlation length never exceeds the interatomic distance, even at T=0. The static structure factor becomes dispersive, indicating a selection of modes by thermal and quantum fluctuations. We also calculate the magnetic neutron diffraction cross section in two planes of the reciprocal space and we find a very good agreement with neutron experiments performed on Y(Sc)Mn2 and CsNiCrF6.

© 2000 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.61.1149
DOI:
10.1103/PhysRevB.61.1149
PACS:
75.10.Jm, 75.40.-s, 75.50.Ee