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Phys. Rev. B 60, 9801–9809 (1999)

Nuclear spin-spin coupling in La2-xSrxCuO4 studied by stimulated echo decay

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S. Fujiyama*, M. Takigawa, and Y. Ueda
The Institute for Solid State Physics, The University of Tokyo, Roppongi, Minato-ku, Tokyo 106-8666, Japan

T. Suzuki and N. Yamada
Department of Applied Physics and Chemistry, University of Electro-Communications, Tokyo 182-8585, Japan

Received 20 April 1999; published in the issue dated 1 October 1999

We have performed copper nuclear quadrupole resonance experiments in high-temperature superconductors YBa2Cu4O8, YBa2Cu3O7, and La2-xSrxCuO4 (x=0.12 and x=0.15), using the stimulated echo technique which utilizes the rf-pulse sequence π/2-(τ)-π/2-(T-τ)-π/2. The τ and T dependences of the stimulated echo intensity is analyzed by a model that includes the spin-lattice relaxation process (T1 process) and the fluctuating local field due to nuclear spin-spin coupling. The model gives quantitative account of the experimental results in YBa2Cu4O8 and YBa2Cu3O7, using the known values of 1/T1 and 1/T2G, the Gaussian decay rate of the spin-echo intensity. The same model applied to La2-xSrxCuO4 enables us to extract the value of T2G. Our results indicate that T1T/T2Gz shows significant temperature dependence for z=2 but is approximately independent of temperature for z=1. This implies that the dynamic exponent is close to one in La2-xSrxCuO4.

© 1999 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.60.9801
DOI:
10.1103/PhysRevB.60.9801
PACS:
74.25.Nf, 74.72.Dn, 76.60.Lz, 76.60.Gv

*Electronic address: fujiyama@kodama.issp.u-tokyo.ac.jp