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Phys. Rev. B 58, 14462–14466 (1998)

Unexpected behavior of the antiferromagnetic mode of NiO

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M. Grimsditch
Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439

L. E. McNeil
Department of Physics and Astronomy, University of North Carolina at Chapel Hill, Chapel Hill, North Carolina 27599-3255

D. J. Lockwood
Institute for Microstructural Sciences, National Research Council of Canada, Ottawa, Ontario, Canada, K1A OR6

Received 19 December 1997; published in the issue dated 1 December 1998

Although NiO is often considered the classic example of an antiferromagnetic insulator, recent investigations have revealed unexplained features of the magnon spectrum. The present study of the temperature and polarization behavior of first-order magnetic Raman scattering reveals that the polarization selection rules are not described by the generally accepted antisymmetric scattering tensor. The inclusion of quadratic magneto-optic coupling terms can explain the symmetry of the scattering tensor, but does not lead to results consistent with the accepted [112] spin alignment direction.

© 1998 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.58.14462
DOI:
10.1103/PhysRevB.58.14462
PACS:
76.50.+q, 75.50.Ee, 78.30.Hv