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Phys. Rev. B 58, 12758–12769 (1998)

Dynamic exchange-correlation potentials for the electron gas in dimensionality D=3 and D=2

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R. Nifosì, S. Conti*, and M. P. Tosi
Istituto Nazionale di Fisica della Materia and Classe di Scienze, Scuola Normale Superiore, I-56126 Pisa, Italy

Received 12 March 1998; published in the issue dated 15 November 1998

Recent progress in the formulation of a fully dynamical local approximation to time-dependent density functional theory appeals to the longitudinal and transverse components of the exchange and correlation kernel in the linear current-density response of the homogeneous fluid at long wavelength. Both components are evaluated for the electron gas in dimensionality D=3 and D=2 by an approximate decoupling in the equation of motion for the current density, which accounts for processes of excitation of two electron-hole pairs. Each pair is treated in the random phase approximation, but the role of exchange and correlation is also examined; in addition, final-state exchange processes are included phenomenologically so as to satisfy the exactly known high-frequency behaviors of the kernel. The transverse and longitudinal spectra involve the same decay channels and are similar in shape. A two-plasmon threshold in the spectrum for two-pair excitations in D=3 leads to a sharp minimum in the real part of the exchange and correlation kernel at twice the plasma frequency. In D=2 the same mechanism leads to a broad spectral peak and to a broad minimum in the real part of the kernel, as a consequence of the dispersion law of the plasmon vanishing at long wavelength. The numerical results have been fitted to simple analytic functions.

© 1998 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevB.58.12758
DOI:
10.1103/PhysRevB.58.12758
PACS:
71.45.Gm

*Present address: Max-Planck-Institute for Mathematics in the Sciences, D-04103 Leipzig, Germany.